This study explores the adaptability of form and skin to solar radiation, focusing on optimizing the interaction between structure and daylight through the optimization of dynamic façade shading devices. By adjusting the folding angles of these shading devices according to different solar radiation levels, the system can be adjusted to maintain optimal lighting conditions. Inspired by origami technology for its geometric diversity, the design allows complex three-dimensional structures to be built from folded sheets. Computational tools such as Grasshopper, Honeybee and Karamba were used in the study to optimize the window-to-wall ratio, folding angles and structural performance, which were applied to the spatial design of hospital wards and library reading rooms. Genetic algorithms further improved the efficiency of solar energy capture and material use, demonstrating the potential of origami-inspired designs in maximizing light efficiency and structural stability in modern architecture.